IMO, Lord Willin' is their best album lyrically, conceptually, and production wise. It also flows better as an album. The dark, minimalist approach on Hell Hath No Fury is cool, but nothing on it was as great as "Virginia", "Grindin", or several of the other songs on Lord Willin'. Til The Casket Drops attempted to reach for a broader audience, but nothing on it was as appealing as say "When The Last Time". So yeah, Lord Willin' was more well rounded without them going to far in either direction.
Exclusive Audio Footage is dope too. It's probably my second favorite of their's.